Intelligent toys play a significant role in children's daily lives and learning. The work aims to explore how human-computer interaction technology can better adapt to children's learning needs and make intelligent toys play their potential and become effective learning tools. By combing the typical cases of children's intelligent innovative learning toys, the cases were analyzed to refine the commonness and characteristics and deeply explore the relationship between the interactive technology of intelligent toys and children's learning objectives and learning methods, thus discussing how to adapt to human-computer interaction technology in different scenarios and learning purposes. From the perspectives of learning objectives, interactive technology, and design theory, the design recommendations are proposed for innovative learning toys of children, providing a reference for how to design intelligent innovative learning toys for children's learning and education.